Not sure if it's the largest, but it's pretty large, and worthy of mention. According to the press release (mind the useless adjectives), "Kansas State University announced today its use of Tegrity Campus to convert an unprecedented 6,000 recorded classes to enhanced podcasts. K-State plans to have all 6,000 class podcasts available to its students this year, making it by far the education realm's largest podcasting implementation worldwide."
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